Confined optical phonon modes in aligned nanorod arrays detected by resonant inelastic light scattering.

نویسندگان

  • Concetta Nobile
  • Vladimir A Fonoberov
  • Stefan Kudera
  • Antonio Della Torre
  • Antonio Ruffino
  • Gerwin Chilla
  • Tobias Kipp
  • Detlef Heitmann
  • Liberato Manna
  • Roberto Cingolani
  • Alexander A Balandin
  • Roman Krahne
چکیده

We investigated the optical phonon excitations of laterally aligned nanorod arrays by resonant Raman scattering. We observed a strong suppression of the surface-optical phonon modes in the closely packed aligned arrays and a small asymmetry in the longitudinal-optical phonon peak with respect to the rod alignment orientation. These observations can be explained by the spatial distribution of the potential of the different phonon modes derived from the first principles calculations.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Spectroscopy, Structural, and Optical Investigations of NiFe2O4 Ferrite

Ni ferrite crystalline material is synthesized using a sol-gel method at two different temperatures. The vibrational and stretching modes, crystalline phase, size distribution and morphology of the products are investigated via Raman back-scattering and Fourier transform infrared (FTIR) spectroscopy, XRD and FESEM, respectively. Vibrational modes of spinel ferrite are observed at Raman and FTIR...

متن کامل

Interface and confined polar optical phonons in spherical ZnO quantum dots with wurtzite crystal structure

We derive analytically the interface and confined polar optical-phonon modes for spherical quantum dots with wurtzite crystal structure. While the frequency of confined optical phonons in zincblende nanocrystals is equal to that of the bulk crystal phonons, the confined polar optical phonons in wurtzite nanocrystals are shown to have a discrete spectrum of frequencies different from those in bu...

متن کامل

Atomic-scale confinement of resonant optical fields.

In the presence of matter, there is no fundamental limit preventing confinement of visible light even down to atomic scales. Achieving such confinement and the corresponding resonant intensity enhancement inevitably requires simultaneous control over atomic-scale details of material structures and over the optical modes that such structures support. By means of self-assembly we have obtained si...

متن کامل

Disentangling the effects of nanoscale structural variations on the light emission wavelength of single nano-emitters: InGaN/GaN multiquantum well nano-LEDs for a case study.

The scattering in the light emission wavelength of semiconductor nano-emitters assigned to nanoscale variations in strain, thickness, and composition is critical in current and novel nanotechnologies from highly efficient light sources to photovoltaics. Here, we present a correlated experimental and theoretical study of single nanorod light emitting diodes (nano-LEDs) based on InGaN/GaN multiqu...

متن کامل

Extraordinary Optical Reflection from Annular Dielectric Nanorod Arrays

Responses of free standing subwavelength annular dielectric nanorod arrays are described. Extreme reflection peaks with high quality factor follow a multiple scattering approach, which can be explained by geometrical resonance. It is demonstrated that the value and the resonant frequency of the sharp geometric resonance modes can be tuned by geometric parameters such as the outer radius, inner ...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Nano letters

دوره 7 2  شماره 

صفحات  -

تاریخ انتشار 2007